| Posted: Jan 04, 2017 |
Light can switch on atomically thin topological materials
(Nanowerk News) Theoretical physicists at the Department of Energy’s SLAC National Accelerator Laboratory used computer simulations to show how special light pulses could create robust channels where electricity flows without resistance in an atomically thin semiconductor.
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If this approach is confirmed by experiments, it could open the door to a new way of creating and controlling this desirable property in a wider range of materials than is possible today.
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The result was published in Nature Communications ("All-optical materials design of chiral edge modes in transition-metal dichalcogenides").
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| This animation shows the creation and disappearance of conditions that produce paths where electricity can travel with no resistance in a single layer of tungsten disulfide. It’s based on simulations in which the material is illuminated with circularly polarized light whose wavelengths vary from near infrared to red. Each frame is a diagram of the material’s electrons. The thin bright area that gradually appears in the middle of the frame and then disappears signifies the desired conditions. (Martin Claassen/Stanford University)
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Over the past decade, understanding how to create this exotic type of material – known as “topologically protected” because its surface states are impervious to minor distortions – has been a hot research topic in materials science. The best-known examples are topological insulators, which conduct electricity with no resistance in confined channels along their edges or surfaces, but not through their interiors.
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SLAC and Stanford University researchers have been at the forefront of discovering such materials and investigating their properties, which could have future applications in microelectronic circuits and devices. This year’s Nobel Prize in Physics was awarded to three scientists who first suggested the possibility of topologically protected material properties.
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Previous theoretical studies had looked at how light might induce topologically protected phenomena in graphene, a sheet of pure carbon just one atom thick. Unfortunately, it would take an impractically high light energy and intensity to induce that effect in graphene. In this study, SLAC researchers focused on tungsten disulfide and related compounds, which form sheets just one molecule thick and are intrinsically semiconducting.
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The researchers simulated experiments in which pulses of circularly polarized light, in the red to near-infrared wavelength range, hit a single layer of tungsten disulfide. The results showed that during the time the material was illuminated, its electrons organized themselves in a manner fundamentally different from graphene, creating new paths with absolutely no electrical resistance along the sample’s edges.
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| A frame from the above animation shows electron states in a single layer of tungsten disulfide crystal that’s been illuminated with circularly polarized light in the red to near-infrared wavelength range. The thin, bright area in the middle signifies “topologically protected” paths where electricity can travel with no resistance. (Image: Martin Claassen/Stanford University)
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To account for the fluctuating interactions between light waves and electrons, the researchers employed a periodically time-varying frame of reference that had roots dating back to the 1880s and French mathematician Gaston Floquet. The approach clearly showed that lower-energy light, to which the material would seem transparent, would create topologically protected, no-resistance edge paths in the tungsten disulfide monolayer.
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Moreover, the simulation showed that unwanted heating of the material that would disrupt the paths could be avoided by tuning the light energy to be slightly less than the most-efficient "resonant" energy.
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“We are the first to connect first-principles material models with light-induced topologically protected states while mitigating excess material heating,” said Martin Claassen, a Stanford graduate student working at SLAC and lead author of the technical paper.
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The researchers are in discussions with other research groups that could lead to experiments that test their theoretical predictions in real materials.
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