Dec 23, 2020 
Theory describes quantum phenomenon in nanomaterials
(Nanowerk News) Theoretical physicists Yoshimichi Teratani and Akira Oguri of Osaka City University, and Rui Sakano of the University of Tokyo have developed mathematical formulas that describe a physical phenomenon happening within quantum dots and other nanosized materials.

The formulas, published in the journal Physical Review Letters ("Fermi Liquid Theory for Nonlinear Transport through a Multilevel Anderson Impurity"), could be applied to further theoretical research about the physics of quantum dots, ultracold atomic gasses, and quarks.


A schematic illustration of a nanoscale circuit. A quantum dot (the yellow part) is connected to two lead electrodes (the blue parts). Electrons tunneling into the quantum dot from the electrodes interact with each other to form a highly correlated quantum state, called “Fermi liquid”. Both nonlinear electric current passing through the quantum dot and its fluctuations that appear as a noise carry important signals, which can unveil underlying physics of the quantum liquid. It is clarified that threebody correlations of the electrons evolve significantly and play essential roles in the quantum state under the external fields that break the particlehole or timereversal symmetry. (Image: Rui Sakano)

At issue is ‘the Kondo effect’. This effect was first described in 1964 by Japanese theoretical physicist Jun Kondo in some magnetic materials, but now appears to happen in many other systems, including quantum dots and other nanoscale materials.

Normally, electrical resistance drops in metals as the temperature drops. But in metals containing magnetic impurities, this only happens down to a critical temperature, beyond which resistance rises with dropping temperatures.

Scientists were eventually able to show that, at very low temperatures near absolute zero, electron spins become entangled with the magnetic impurities, forming a cloud that screens their magnetism. The cloud’s shape changes with further temperature drops, leading to a rise in resistance. This same effect happens when other external ‘perturbations’, such as a voltage or magnetic field, are applied to the metal.

Teratani, Sakano and Oguri wanted to develop mathematical formulas to describe the evolution of this cloud in quantum dots and other nanoscale materials, which is not an easy task.

To describe such a complex quantum system, they started with a system at absolute zero where a wellestablished theoretical model, namely Fermi liquid theory, for interacting electrons is applicable. They then added a ‘correction’ that describes another aspect of the system against external perturbations. Using this technique, they wrote formulas describing electrical current and its fluctuation through quantum dots.

Their formulas indicate electrons interact within these systems in two different ways that contribute to the Kondo effect. First, two electrons collide with each other, forming welldefined quasiparticles that propagate within the Kondo cloud. More significantly, an interaction called a threebody contribution occurs. This is when two electrons combine in the presence of a third electron, causing an energy shift of quasiparticles.

“The formulas’ predictions could soon be investigated experimentally”, Oguri says. “Studies along the lines of this research have only just begun,” he adds.

The formulas could also be extended to understand other quantum phenomena, such as quantum particle movement through quantum dots connected to superconductors. Quantum dots could be a key for realizing quantum information technologies, such as quantum computers and quantum communication.
